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The buses, ________ were already full, were surrounded by an angry crowd.

A.most of them B.which most
C.most of which D.that most

C

解析试题分析:考查非限制性定语从句。根据逗号判断,句子是非限制性定语从句,most of...意为“......的大多数”,排除B、D;A项不能引导从句,如果在逗号后添加and,则句子变成两个并列的分句。目前来看,句子是主从复合句,most of which指代大多数公交车,故选C。
考点:考查非限制性定语从句

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